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Degradation of 4-nitrophenol (4-NP) using Fe-TiO2 as a heterogeneous photo-Fenton catalyst.
J Hazard Mater. 2010 Apr 15; 176(1-3):569-74.JH

Abstract

Photocatalytic degradation of 4-nitrophenol was investigated using Fe-doped (1, 3, 5 and 8 wt.% Fe) TiO(2) catalysts under UV light irradiation in aqueous dispersions in the presence of H(2)O(2). Photocatalysts with the lowest Fe content (1%) showed a considerably better behavior with respect to the unloaded TiO(2) and the catalysts with higher Fe contents. Photocatalytic degradation was studied under different conditions such as amounts of 1% Fe-TiO(2) catalyst, H(2)O(2) dose and initial pH of 4-NP solution. The results indicated that about 67.53% total organic carbon of a solution containing 20 mg L(-1) 4-NP was removed at pH 6.17 by using 4.9 mM of H(2)O(2) and 0.4 g L(-1) of the catalyst in a 2-L batch photo-reactor, the complete degradation of 4-NP occurring after 60 min. It was also observed that catalytic behavior could be reproduced in consecutive experiments without a considerable decrease of the UV/Fe-TiO(2)/H(2)O(2) process efficiency.

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Authors+Show Affiliations

Zhao B
College of Chemical Engineering, Northwest University, 229 Taibai North Road, Xi'an, Shaanxi 710069, China. zxlbx@china.com
Mele G
No affiliation info available
Pio I
No affiliation info available
Li J
No affiliation info available
Palmisano L
No affiliation info available
Vasapollo G
No affiliation info available

MeSH

CatalysisHydrogen PeroxideIronNitrophenolsPhotolysisTitaniumUltraviolet Rays

Pub Type(s)

Journal Article

Language

eng

PubMed ID

20004519

Citation

Zhao, Binxia, et al. "Degradation of 4-nitrophenol (4-NP) Using Fe-TiO2 as a Heterogeneous photo-Fenton Catalyst." Journal of Hazardous Materials, vol. 176, no. 1-3, 2010, pp. 569-74.
Zhao B, Mele G, Pio I, et al. Degradation of 4-nitrophenol (4-NP) using Fe-TiO2 as a heterogeneous photo-Fenton catalyst. J Hazard Mater. 2010;176(1-3):569-74.
Zhao, B., Mele, G., Pio, I., Li, J., Palmisano, L., & Vasapollo, G. (2010). Degradation of 4-nitrophenol (4-NP) using Fe-TiO2 as a heterogeneous photo-Fenton catalyst. Journal of Hazardous Materials, 176(1-3), 569-74. https://doi.org/10.1016/j.jhazmat.2009.11.066
Zhao B, et al. Degradation of 4-nitrophenol (4-NP) Using Fe-TiO2 as a Heterogeneous photo-Fenton Catalyst. J Hazard Mater. 2010 Apr 15;176(1-3):569-74. PubMed PMID: 20004519.
* Article titles in AMA citation format should be in sentence-case
TY - JOUR T1 - Degradation of 4-nitrophenol (4-NP) using Fe-TiO2 as a heterogeneous photo-Fenton catalyst. AU - Zhao,Binxia, AU - Mele,Giuseppe, AU - Pio,Iolanda, AU - Li,Jun, AU - Palmisano,Leonardo, AU - Vasapollo,Giuseppe, Y1 - 2009/11/18/ PY - 2009/06/17/received PY - 2009/11/06/revised PY - 2009/11/10/accepted PY - 2009/12/17/entrez PY - 2009/12/17/pubmed PY - 2010/5/19/medline SP - 569 EP - 74 JF - Journal of hazardous materials JO - J Hazard Mater VL - 176 IS - 1-3 N2 - Photocatalytic degradation of 4-nitrophenol was investigated using Fe-doped (1, 3, 5 and 8 wt.% Fe) TiO(2) catalysts under UV light irradiation in aqueous dispersions in the presence of H(2)O(2). Photocatalysts with the lowest Fe content (1%) showed a considerably better behavior with respect to the unloaded TiO(2) and the catalysts with higher Fe contents. Photocatalytic degradation was studied under different conditions such as amounts of 1% Fe-TiO(2) catalyst, H(2)O(2) dose and initial pH of 4-NP solution. The results indicated that about 67.53% total organic carbon of a solution containing 20 mg L(-1) 4-NP was removed at pH 6.17 by using 4.9 mM of H(2)O(2) and 0.4 g L(-1) of the catalyst in a 2-L batch photo-reactor, the complete degradation of 4-NP occurring after 60 min. It was also observed that catalytic behavior could be reproduced in consecutive experiments without a considerable decrease of the UV/Fe-TiO(2)/H(2)O(2) process efficiency. SN - 1873-3336 UR - https://www.unboundmedicine.com/medline/citation/20004519/Degradation_of_4_nitrophenol__4_NP__using_Fe_TiO2_as_a_heterogeneous_photo_Fenton_catalyst_ L2 - https://linkinghub.elsevier.com/retrieve/pii/S0304-3894(09)01864-0 DB - PRIME DP - Unbound Medicine ER -