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Degradation efficiencies of azo dye Acid Orange 7 by the interaction of heat, UV and anions with common oxidants: persulfate, peroxymonosulfate and hydrogen peroxide.
J Hazard Mater. 2010 Jul 15; 179(1-3):552-8.JH

Abstract

In this paper, the degradation of azo dye Acid Orange 7 (AO7) by three common peroxides (persulfate (PS), peroxymonosulfate (PMS) or hydrogen peroxide (H(2)O(2))) under various activation conditions, i.e., heat (25-80 degrees C), UV light (254 nm), or anions (SO(4)(2-), NO(3)(-), CO(3)(2-), HCO(3)(-), HPO(4)(2-), and Cl(-)), was investigated. The order of AO7 degradation efficiencies by heat activation is PS>>PMS>H(2)O(2). PS oxidation activated by heat (>50 degrees C) is an effective degradation technology, while PMS and H(2)O(2) are hardly activated. When assisted by UV, peroxides could all be activated and degrade AO7 quickly. The order is PS>H(2)O(2)>PMS. We activated peroxides, for the first time, by using some anions and compared the subsequently degradation efficiencies of AO7. It was found that PMS could be activated by some anions, but PS and H(2)O(2) cannot. The activation efficiencies of PMS by SO(4)(2-) and NO(3)(-) are negligible, whereas remarkable by HCO(3)(-), HPO(4)(2-), Cl(-) and CO(3)(2-). For HCO(3)(-), HPO(4)(2-) and Cl(-), the activation efficiencies become higher with the increase of anion concentration. For CO(3)(2-), however, the activation efficiency is higher at lower concentration.

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Authors+Show Affiliations

Yang S
Key Laboratory of Marine Environment and Ecology, Ministry of Education, Qingdao 266100, China. shiningpup@hotmail.com
Wang P
No affiliation info available
Yang X
No affiliation info available
Shan L
No affiliation info available
Zhang W
No affiliation info available
Shao X
No affiliation info available
Niu R
No affiliation info available

MeSH

AnionsAzo CompoundsBenzenesulfonatesHot TemperatureHydrogen PeroxideHydrogen-Ion ConcentrationIndicators and ReagentsIndustrial WasteOxidantsPeroxidesPotassium CompoundsSpectrophotometry, UltravioletSulfatesSulfuric AcidsTemperatureUltraviolet RaysWaste Disposal, Fluid

Pub Type(s)

Journal Article

Language

eng

PubMed ID

20371151

Citation

Yang, Shiying, et al. "Degradation Efficiencies of Azo Dye Acid Orange 7 By the Interaction of Heat, UV and Anions With Common Oxidants: Persulfate, Peroxymonosulfate and Hydrogen Peroxide." Journal of Hazardous Materials, vol. 179, no. 1-3, 2010, pp. 552-8.
Yang S, Wang P, Yang X, et al. Degradation efficiencies of azo dye Acid Orange 7 by the interaction of heat, UV and anions with common oxidants: persulfate, peroxymonosulfate and hydrogen peroxide. J Hazard Mater. 2010;179(1-3):552-8.
Yang, S., Wang, P., Yang, X., Shan, L., Zhang, W., Shao, X., & Niu, R. (2010). Degradation efficiencies of azo dye Acid Orange 7 by the interaction of heat, UV and anions with common oxidants: persulfate, peroxymonosulfate and hydrogen peroxide. Journal of Hazardous Materials, 179(1-3), 552-8. https://doi.org/10.1016/j.jhazmat.2010.03.039
Yang S, et al. Degradation Efficiencies of Azo Dye Acid Orange 7 By the Interaction of Heat, UV and Anions With Common Oxidants: Persulfate, Peroxymonosulfate and Hydrogen Peroxide. J Hazard Mater. 2010 Jul 15;179(1-3):552-8. PubMed PMID: 20371151.
* Article titles in AMA citation format should be in sentence-case
TY - JOUR T1 - Degradation efficiencies of azo dye Acid Orange 7 by the interaction of heat, UV and anions with common oxidants: persulfate, peroxymonosulfate and hydrogen peroxide. AU - Yang,Shiying, AU - Wang,Ping, AU - Yang,Xin, AU - Shan,Liang, AU - Zhang,Wenyi, AU - Shao,Xueting, AU - Niu,Rui, Y1 - 2010/03/15/ PY - 2009/11/06/received PY - 2010/02/05/revised PY - 2010/03/08/accepted PY - 2010/4/8/entrez PY - 2010/4/8/pubmed PY - 2010/8/13/medline SP - 552 EP - 8 JF - Journal of hazardous materials JO - J Hazard Mater VL - 179 IS - 1-3 N2 - In this paper, the degradation of azo dye Acid Orange 7 (AO7) by three common peroxides (persulfate (PS), peroxymonosulfate (PMS) or hydrogen peroxide (H(2)O(2))) under various activation conditions, i.e., heat (25-80 degrees C), UV light (254 nm), or anions (SO(4)(2-), NO(3)(-), CO(3)(2-), HCO(3)(-), HPO(4)(2-), and Cl(-)), was investigated. The order of AO7 degradation efficiencies by heat activation is PS>>PMS>H(2)O(2). PS oxidation activated by heat (>50 degrees C) is an effective degradation technology, while PMS and H(2)O(2) are hardly activated. When assisted by UV, peroxides could all be activated and degrade AO7 quickly. The order is PS>H(2)O(2)>PMS. We activated peroxides, for the first time, by using some anions and compared the subsequently degradation efficiencies of AO7. It was found that PMS could be activated by some anions, but PS and H(2)O(2) cannot. The activation efficiencies of PMS by SO(4)(2-) and NO(3)(-) are negligible, whereas remarkable by HCO(3)(-), HPO(4)(2-), Cl(-) and CO(3)(2-). For HCO(3)(-), HPO(4)(2-) and Cl(-), the activation efficiencies become higher with the increase of anion concentration. For CO(3)(2-), however, the activation efficiency is higher at lower concentration. SN - 1873-3336 UR - https://www.unboundmedicine.com/medline/citation/20371151/Degradation_efficiencies_of_azo_dye_Acid_Orange_7_by_the_interaction_of_heat_UV_and_anions_with_common_oxidants:_persulfate_peroxymonosulfate_and_hydrogen_peroxide_ L2 - https://linkinghub.elsevier.com/retrieve/pii/S0304-3894(10)00345-6 DB - PRIME DP - Unbound Medicine ER -