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Roll-to-Roll Gravure Printed Electrochemical Sensors for Wearable and Medical Devices.
ACS Nano. 2018 07 24; 12(7):6978-6987.AN

Abstract

As recent developments in noninvasive biosensors spearhead the thrust toward personalized health and fitness monitoring, there is a need for high throughput, cost-effective fabrication of flexible sensing components. Toward this goal, we present roll-to-roll (R2R) gravure printed electrodes that are robust under a range of electrochemical sensing applications. We use inks and electrode morphologies designed for electrochemical and mechanical stability, achieving devices with uniform redox kinetics printed on 150 m flexible substrate rolls. We show that these electrodes can be functionalized into consistently high performing sensors for detecting ions, metabolites, heavy metals, and other small molecules in noninvasively accessed biofluids, including sensors for real-time, in situ perspiration monitoring during exercise. This development of robust and versatile R2R gravure printed electrodes represents a key translational step in enabling large-scale, low-cost fabrication of disposable wearable sensors for personalized health monitoring applications.

Authors+Show Affiliations

Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Printed Electronics Engineering , Sunchon National University , Sunchon , Jeonnam 540-742 , South Korea.Department of Printed Electronics Engineering , Sunchon National University , Sunchon , Jeonnam 540-742 , South Korea.Department of Printed Electronics Engineering , Sunchon National University , Sunchon , Jeonnam 540-742 , South Korea.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.Department of Printed Electronics Engineering , Sunchon National University , Sunchon , Jeonnam 540-742 , South Korea.Department of Electrical Engineering and Computer Sciences , University of California , Berkeley , California 94720 , United States. Berkeley Sensor and Actuator Center , University of California , Berkeley , California 94720 , United States. Materials Sciences Division , Lawrence Berkeley National Laboratory , Berkeley , California 94720 , United States.

Pub Type(s)

Journal Article
Research Support, Non-U.S. Gov't
Research Support, U.S. Gov't, Non-P.H.S.

Language

eng

PubMed ID

29924589

Citation

Bariya, Mallika, et al. "Roll-to-Roll Gravure Printed Electrochemical Sensors for Wearable and Medical Devices." ACS Nano, vol. 12, no. 7, 2018, pp. 6978-6987.
Bariya M, Shahpar Z, Park H, et al. Roll-to-Roll Gravure Printed Electrochemical Sensors for Wearable and Medical Devices. ACS Nano. 2018;12(7):6978-6987.
Bariya, M., Shahpar, Z., Park, H., Sun, J., Jung, Y., Gao, W., Nyein, H. Y. Y., Liaw, T. S., Tai, L. C., Ngo, Q. P., Chao, M., Zhao, Y., Hettick, M., Cho, G., & Javey, A. (2018). Roll-to-Roll Gravure Printed Electrochemical Sensors for Wearable and Medical Devices. ACS Nano, 12(7), 6978-6987. https://doi.org/10.1021/acsnano.8b02505
Bariya M, et al. Roll-to-Roll Gravure Printed Electrochemical Sensors for Wearable and Medical Devices. ACS Nano. 2018 07 24;12(7):6978-6987. PubMed PMID: 29924589.
* Article titles in AMA citation format should be in sentence-case
TY - JOUR T1 - Roll-to-Roll Gravure Printed Electrochemical Sensors for Wearable and Medical Devices. AU - Bariya,Mallika, AU - Shahpar,Ziba, AU - Park,Hyejin, AU - Sun,Junfeng, AU - Jung,Younsu, AU - Gao,Wei, AU - Nyein,Hnin Yin Yin, AU - Liaw,Tiffany Sun, AU - Tai,Li-Chia, AU - Ngo,Quynh P, AU - Chao,Minghan, AU - Zhao,Yingbo, AU - Hettick,Mark, AU - Cho,Gyoujin, AU - Javey,Ali, Y1 - 2018/06/25/ PY - 2018/6/21/pubmed PY - 2019/10/1/medline PY - 2018/6/21/entrez KW - flexible electronics KW - gravure printing KW - in situ analysis KW - multiplexed sensing KW - roll-to-roll processing KW - wearable biosensors SP - 6978 EP - 6987 JF - ACS nano JO - ACS Nano VL - 12 IS - 7 N2 - As recent developments in noninvasive biosensors spearhead the thrust toward personalized health and fitness monitoring, there is a need for high throughput, cost-effective fabrication of flexible sensing components. Toward this goal, we present roll-to-roll (R2R) gravure printed electrodes that are robust under a range of electrochemical sensing applications. We use inks and electrode morphologies designed for electrochemical and mechanical stability, achieving devices with uniform redox kinetics printed on 150 m flexible substrate rolls. We show that these electrodes can be functionalized into consistently high performing sensors for detecting ions, metabolites, heavy metals, and other small molecules in noninvasively accessed biofluids, including sensors for real-time, in situ perspiration monitoring during exercise. This development of robust and versatile R2R gravure printed electrodes represents a key translational step in enabling large-scale, low-cost fabrication of disposable wearable sensors for personalized health monitoring applications. SN - 1936-086X UR - https://www.unboundmedicine.com/medline/citation/29924589/Roll_to_Roll_Gravure_Printed_Electrochemical_Sensors_for_Wearable_and_Medical_Devices_ L2 - https://dx.doi.org/10.1021/acsnano.8b02505 DB - PRIME DP - Unbound Medicine ER -