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Microwave-Assisted Synthesis of CuS Hierarchical Nanosheets as the Cathode Material for High-Capacity Rechargeable Magnesium Batteries.
ACS Appl Mater Interfaces. 2019 Feb 20; 11(7):7046-7054.AA

Abstract

Rechargeable magnesium batteries (rMBs) have been recognized as one of most promising next-generation energy storage devices with high energy and power density. However, the development of rMBs has been hampered by the lack of usable cathode materials with high capacity and cycling stability. Herein, we report an ultra-rapid, cost-effective, and scalable synthesis of ultrathin CuS hierarchical nanosheets by a one-step microwave-assisted preparation. Benefiting from the exceptional structural configuration, when used as the cathode material for rMBs at room temperature, the CuS hierarchical nanosheets deliver a high reversible discharge capacity of 300 mA h g-1 at 20 mA g-1, remarkable rate capability (256.5 mA h g-1 at 50 mA g-1 and 237.5 mA h g-1 at 100 mA g-1), and excellent cycling stability (135 mA h g-1 at 200 mA g-1 over 200 cycles). To date, the obtained excellent electrochemical performances are superior to most results ever reported for cathode materials of rMBs.

Authors+Show Affiliations

Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications , Beijing Institute of Technology , Beijing 100081 , China.

Pub Type(s)

Journal Article

Language

eng

PubMed ID

30667214

Citation

Wang, Zhitao, et al. "Microwave-Assisted Synthesis of CuS Hierarchical Nanosheets as the Cathode Material for High-Capacity Rechargeable Magnesium Batteries." ACS Applied Materials & Interfaces, vol. 11, no. 7, 2019, pp. 7046-7054.
Wang Z, Rafai S, Qiao C, et al. Microwave-Assisted Synthesis of CuS Hierarchical Nanosheets as the Cathode Material for High-Capacity Rechargeable Magnesium Batteries. ACS Appl Mater Interfaces. 2019;11(7):7046-7054.
Wang, Z., Rafai, S., Qiao, C., Jia, J., Zhu, Y., Ma, X., & Cao, C. (2019). Microwave-Assisted Synthesis of CuS Hierarchical Nanosheets as the Cathode Material for High-Capacity Rechargeable Magnesium Batteries. ACS Applied Materials & Interfaces, 11(7), 7046-7054. https://doi.org/10.1021/acsami.8b20533
Wang Z, et al. Microwave-Assisted Synthesis of CuS Hierarchical Nanosheets as the Cathode Material for High-Capacity Rechargeable Magnesium Batteries. ACS Appl Mater Interfaces. 2019 Feb 20;11(7):7046-7054. PubMed PMID: 30667214.
* Article titles in AMA citation format should be in sentence-case
TY - JOUR T1 - Microwave-Assisted Synthesis of CuS Hierarchical Nanosheets as the Cathode Material for High-Capacity Rechargeable Magnesium Batteries. AU - Wang,Zhitao, AU - Rafai,Souleymen, AU - Qiao,Chen, AU - Jia,Jian, AU - Zhu,Youqi, AU - Ma,Xilan, AU - Cao,Chuanbao, Y1 - 2019/02/05/ PY - 2019/1/23/pubmed PY - 2019/1/23/medline PY - 2019/1/23/entrez KW - CuS hierarchical nanosheets KW - cathode KW - high capacity KW - microwave-assisted synthesis KW - rechargeable magnesium batteries SP - 7046 EP - 7054 JF - ACS applied materials & interfaces JO - ACS Appl Mater Interfaces VL - 11 IS - 7 N2 - Rechargeable magnesium batteries (rMBs) have been recognized as one of most promising next-generation energy storage devices with high energy and power density. However, the development of rMBs has been hampered by the lack of usable cathode materials with high capacity and cycling stability. Herein, we report an ultra-rapid, cost-effective, and scalable synthesis of ultrathin CuS hierarchical nanosheets by a one-step microwave-assisted preparation. Benefiting from the exceptional structural configuration, when used as the cathode material for rMBs at room temperature, the CuS hierarchical nanosheets deliver a high reversible discharge capacity of 300 mA h g-1 at 20 mA g-1, remarkable rate capability (256.5 mA h g-1 at 50 mA g-1 and 237.5 mA h g-1 at 100 mA g-1), and excellent cycling stability (135 mA h g-1 at 200 mA g-1 over 200 cycles). To date, the obtained excellent electrochemical performances are superior to most results ever reported for cathode materials of rMBs. SN - 1944-8252 UR - https://www.unboundmedicine.com/medline/citation/30667214/Microwave_Assisted_Synthesis_of_CuS_Hierarchical_Nanosheets_as_the_Cathode_Material_for_High_Capacity_Rechargeable_Magnesium_Batteries_ L2 - https://dx.doi.org/10.1021/acsami.8b20533 DB - PRIME DP - Unbound Medicine ER -
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