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Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook.
ACS Appl Mater Interfaces. 2019 Jun 26; 11(25):22029-22050.AA

Abstract

All-solid-state batteries (ASSBs) based on inorganic solid electrolytes promise improved safety, higher energy density, longer cycle life, and lower cost than conventional Li-ion batteries. However, their practical application is hampered by the high resistance arising at the solid-solid electrode-electrolyte interface. Although the exact mechanism of this interface resistance has not been fully understood, various chemical, electrochemical, and chemo-mechanical processes govern the charge transfer phenomenon at the interface. This paper reports the interfacial behavior of the lithium and the cathode in oxide and sulfide inorganic solid-electrolytes and how that affects the overall battery performance. An overview of the recent reports dealing with high resistance at the anodic and cathodic interfaces is presented and the scientific and engineering aspects of the approaches adopted to solve the issue are summarized.

Authors+Show Affiliations

Helmholtz Institute Ulm , Helmholtzstraβe, 11 , Ulm 89081 , Germany.Helmholtz Institute Ulm , Helmholtzstraβe, 11 , Ulm 89081 , Germany.Department of Chemistry , University of Calgary , 2500 University Drive Northwest , Calgary , Alberta T2N 1N4 , Canada.Helmholtz Institute Ulm , Helmholtzstraβe, 11 , Ulm 89081 , Germany.

Pub Type(s)

Journal Article

Language

eng

PubMed ID

31144798

Citation

Pervez, Syed Atif, et al. "Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook." ACS Applied Materials & Interfaces, vol. 11, no. 25, 2019, pp. 22029-22050.
Pervez SA, Cambaz MA, Thangadurai V, et al. Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook. ACS Appl Mater Interfaces. 2019;11(25):22029-22050.
Pervez, S. A., Cambaz, M. A., Thangadurai, V., & Fichtner, M. (2019). Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook. ACS Applied Materials & Interfaces, 11(25), 22029-22050. https://doi.org/10.1021/acsami.9b02675
Pervez SA, et al. Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook. ACS Appl Mater Interfaces. 2019 Jun 26;11(25):22029-22050. PubMed PMID: 31144798.
* Article titles in AMA citation format should be in sentence-case
TY - JOUR T1 - Interface in Solid-State Lithium Battery: Challenges, Progress, and Outlook. AU - Pervez,Syed Atif, AU - Cambaz,Musa Ali, AU - Thangadurai,Venkataraman, AU - Fichtner,Maximilian, Y1 - 2019/06/13/ PY - 2019/5/31/pubmed PY - 2019/5/31/medline PY - 2019/5/31/entrez KW - Li dendrites KW - interface resistance KW - interfacial characterization KW - solid-electrolyte KW - solid-state battery SP - 22029 EP - 22050 JF - ACS applied materials & interfaces JO - ACS Appl Mater Interfaces VL - 11 IS - 25 N2 - All-solid-state batteries (ASSBs) based on inorganic solid electrolytes promise improved safety, higher energy density, longer cycle life, and lower cost than conventional Li-ion batteries. However, their practical application is hampered by the high resistance arising at the solid-solid electrode-electrolyte interface. Although the exact mechanism of this interface resistance has not been fully understood, various chemical, electrochemical, and chemo-mechanical processes govern the charge transfer phenomenon at the interface. This paper reports the interfacial behavior of the lithium and the cathode in oxide and sulfide inorganic solid-electrolytes and how that affects the overall battery performance. An overview of the recent reports dealing with high resistance at the anodic and cathodic interfaces is presented and the scientific and engineering aspects of the approaches adopted to solve the issue are summarized. SN - 1944-8252 UR - https://www.unboundmedicine.com/medline/citation/31144798/Interface_in_Solid_State_Lithium_Battery:_Challenges_Progress_and_Outlook_ L2 - https://dx.doi.org/10.1021/acsami.9b02675 DB - PRIME DP - Unbound Medicine ER -
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