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Structural Engineering of Low-Dimensional Metal-Organic Frameworks: Synthesis, Properties, and Applications.
Adv Sci (Weinh) 2019; 6(12):1802373AS

Abstract

Low-dimensional metal-organic frameworks (LD MOFs) have attracted increasing attention in recent years, which successfully combine the unique properties of MOFs, e.g., large surface area, tailorable structure, and uniform cavity, with the distinctive physical and chemical properties of LD nanomaterials, e.g., high aspect ratio, abundant accessible active sites, and flexibility. Significant progress has been made in the morphological and structural regulation of LD MOFs in recent years. It is still of great significance to further explore the synthetic principles and dimensional-dependent properties of LD MOFs. In this review, recent progress in the synthesis of LD MOF-based materials and their applications are summarized, with an emphasis on the distinctive advantages of LD MOFs over their bulk counterparties. First, the unique physical and chemical properties of LD MOF-based materials are briefly introduced. Synthetic strategies of various LD MOFs, including 1D MOFs, 2D MOFs, and LD MOF-based composites, as well as their derivatives, are then summarized. Furthermore, the potential applications of LD MOF-based materials in catalysis, energy storage, gas adsorption and separation, and sensing are introduced. Finally, challenges and opportunities of this fascinating research field are proposed.

Authors+Show Affiliations

College of Materials Science and Engineering Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310014 P. R. China.College of Materials Science and Engineering Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310014 P. R. China.College of Materials Science and Engineering Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310014 P. R. China.College of Materials Science and Engineering Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310014 P. R. China.Center for Membrane Separation and Water Science & Technology Ocean College Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310014 P. R. China. Huzhou Institute of Collaborative Innovation Center for Membrane Separation and Water Treatment Zhejiang University of Technology Huzhou Zhejiang 313000 P. R. China.College of Materials Science and Engineering Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310014 P. R. China. State Key Laboratory Breeding Base of Green Chemistry Synthesis Technology Zhejiang University of Technology 18 Chaowang Road Hangzhou Zhejiang 310032 P. R. China.

Pub Type(s)

Journal Article
Review

Language

eng

PubMed ID

31380160

Citation

Liu, Wenxian, et al. "Structural Engineering of Low-Dimensional Metal-Organic Frameworks: Synthesis, Properties, and Applications." Advanced Science (Weinheim, Baden-Wurttemberg, Germany), vol. 6, no. 12, 2019, p. 1802373.
Liu W, Yin R, Xu X, et al. Structural Engineering of Low-Dimensional Metal-Organic Frameworks: Synthesis, Properties, and Applications. Adv Sci (Weinh). 2019;6(12):1802373.
Liu, W., Yin, R., Xu, X., Zhang, L., Shi, W., & Cao, X. (2019). Structural Engineering of Low-Dimensional Metal-Organic Frameworks: Synthesis, Properties, and Applications. Advanced Science (Weinheim, Baden-Wurttemberg, Germany), 6(12), p. 1802373. doi:10.1002/advs.201802373.
Liu W, et al. Structural Engineering of Low-Dimensional Metal-Organic Frameworks: Synthesis, Properties, and Applications. Adv Sci (Weinh). 2019 Jun 19;6(12):1802373. PubMed PMID: 31380160.
* Article titles in AMA citation format should be in sentence-case
TY - JOUR T1 - Structural Engineering of Low-Dimensional Metal-Organic Frameworks: Synthesis, Properties, and Applications. AU - Liu,Wenxian, AU - Yin,Ruilian, AU - Xu,Xilian, AU - Zhang,Lin, AU - Shi,Wenhui, AU - Cao,Xiehong, Y1 - 2019/04/18/ PY - 2018/12/31/received PY - 2019/03/13/revised PY - 2019/8/6/entrez PY - 2019/8/6/pubmed PY - 2019/8/6/medline KW - catalysts KW - electrode materials KW - low‐dimensional nanomaterials KW - metal–organic frameworks KW - sensors SP - 1802373 EP - 1802373 JF - Advanced science (Weinheim, Baden-Wurttemberg, Germany) JO - Adv Sci (Weinh) VL - 6 IS - 12 N2 - Low-dimensional metal-organic frameworks (LD MOFs) have attracted increasing attention in recent years, which successfully combine the unique properties of MOFs, e.g., large surface area, tailorable structure, and uniform cavity, with the distinctive physical and chemical properties of LD nanomaterials, e.g., high aspect ratio, abundant accessible active sites, and flexibility. Significant progress has been made in the morphological and structural regulation of LD MOFs in recent years. It is still of great significance to further explore the synthetic principles and dimensional-dependent properties of LD MOFs. In this review, recent progress in the synthesis of LD MOF-based materials and their applications are summarized, with an emphasis on the distinctive advantages of LD MOFs over their bulk counterparties. First, the unique physical and chemical properties of LD MOF-based materials are briefly introduced. Synthetic strategies of various LD MOFs, including 1D MOFs, 2D MOFs, and LD MOF-based composites, as well as their derivatives, are then summarized. Furthermore, the potential applications of LD MOF-based materials in catalysis, energy storage, gas adsorption and separation, and sensing are introduced. Finally, challenges and opportunities of this fascinating research field are proposed. SN - 2198-3844 UR - https://www.unboundmedicine.com/medline/citation/31380160/Structural_Engineering_of_Low_Dimensional_Metal_Organic_Frameworks:_Synthesis_Properties_and_Applications_ L2 - https://www.ncbi.nlm.nih.gov/pmc/articles/pmid/31380160/ DB - PRIME DP - Unbound Medicine ER -